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I liked all the tier 2 sets, I think they were some of the best looking sets that have been designed. Although if I had to pick one I would have to go with the Paladin teir 2 set Judgement.
One of my favorites would be Vestments of Absolution (priest tier 6), It just says: "I decide if you will live or die."
T2. Nothing beat killing Nef and getting my 8 pc.
Despite how it looked from the back, I loved the Priest Tier 8. The wings-of-light effect was striking, and everything just screamed "holy healer".Warriors' Tier 2 is a close second. Nothing like blades, blades everywhere.
My favorite tier set was the Warlock Tier 1 set (Felheart Raiment). I think it really captures the flavor and essence of what the early Warlocks were like and how they viewed the world through the eyes of their demon familiars.
Judgement, Paladin Tier 2, was definitely the coolest Tier set of all time.
Paladin T2. Reason being because it is the most iconic Tier set of the entire game, and is perfectly suited to the Paladin class. The whole holy Justicar feeling to it really is awesome :)
Out of all the sets I have used, Paladin T9 was my favourite. No dresses (because paladins shouldn't be made to wear dresses). I liked the gold and blue highlights on the Alliance armour, they looked awesome on my draenei. The red and gold for the Horde armour was good for my blood elf too.
The Twin Blades of Azzinoth, its not really a tier set, but they're the most awesome set ingame!
Without a doubt it would have to be Season 2 Pvp Lock set http://www.wowhead.com/itemset=702..I think this gear is some of the best gear in the game and it lets me reminisce about the Best time of the Game being BC
Druid T10 HeroicSanctified Lasherweave Garb is my personal favorite tier set. While the set bonuses were rather weak, the item art is what makes it amazing. The giant tooth shoulders and vine-horned helm combined with the brown, green, and purple color scheme made any druid wearing this worthy of vanquishing Arthas.
The hunter's tier 11.Because it look's like a murloc.A MURLOC. Nothing can be more victorious.
Definitely T6 and most especially my priest raid gear! I love the all over look. With the bound and blindfolded woman on the shoulders (hot), the halo around the hood, and the overall sleek look of the set this was definitely my favorite thus far fulfilling all my shiny needs!